Must read: Organic semiconductors

We are delighted to share a selection of “must read” articles published in RSC Applied Interfaces in the field of organic semiconductors. The articles explore the application of organic semiconductor materials in photovoltaics, transistors, neuromorphic computing, and sensing. 

Organic photovoltaics 

There are different strategies to improve organic photovoltaic performance through interface engineering. The papers below show how the charge-state formation at interfaces affect charge-transfer properties and ultimately device performance, as well as more sustainable processing methods. 

            Solution treatment controls charge-transfer states and energy-level alignment at hybrid CuSCN-organic interfaces 

Yingying Li, Zhewei Chen, Wenjie Zhou, Qi Wang, Yuan Zhang, Tao Song, Baoquan Sun, Steffen Duhm 

  All slot-die coated organic solar cells using an amine processed cathode interlayer based upon an amino acid functionalised perylene bisimide 

Rebecca E. Ginesi, Muhammad R. Niazi, Gregory C. Welch, Emily R. Draper 

  Dielectric-constant effects on the exciton dissociation and photovoltaic conversion efficiency of water-soluble green conducting polymers 

Xin Wei, Daniel Williams, Giovanni Fanchini 

 

Organic transistors for neuromorphic computing  

These studies explore organic transistor devices that reproduce aspects of neural and synaptic behaviour. They examine how operating voltage and material properties such as polymer molecular weight and film thickness affect the speed and dynamics of neuromorphic devices. 

  Voltage-dependent time constants for neuromorphic organic electrochemical transistor applications 

Shunsuke Yamamoto, Nanako Kanazumi, Masaya Mitsuishi 

  Exploring response time and synaptic plasticity in P3HT ion-gated transistors for neuromorphic computing: impact of P3HT molecular weight and film thickness 

Ramin Karimi Azari, Zhaojing Gao, Alexandre Carrière, Clara Santato 

 

Organic semiconductors as sensors 

These papers focus on functional sensing devices made using flexible or scalable electronic materials, highlighting practical device functionality and manufacturing scalability. 

  Flexible strain sensors based on silver nanowires and UV-curable acrylate elastomers for wrist movement monitoring 

Shuhao Li, Wenjin Wu, Yu Chang, Weiquan Chen, Yijie Liu, Zifeng He, Yan Pu, Ivan S. Babichuk, Terry Tao Ye, Zhaoli Gao, Jian Yang 

  Bias switchable narrowband/broadband NIR organic photodetector fabricated with a scalable technique 

Lai-Hung Lai, Wei-Hsiang Lin, Chin-Chuan Hsieh, Maria Antonietta Loi 

 

Thin film optimisation  

The articles below explore how important it is to optimise the molecule structure of organic semiconductor materials to enhance their performance. Molecular design, polymer structure and thin-film organisation all influence application-relevant properties like charge mobility. These studies highlight the need to balance electrical performance and other desirable properties like stretchability or stability. 

  Anisotropic charge transport study of highly oriented P4T2F-HD thin film fabricated at air–liquid interface through second harmonic generation (SHG) analysis 

Radhe Shyam, Takaaki Manaka, Rajiv Prakash 

  N-type semiconducting polymers with an improved isotropic mobility–stretchability stability by using structural isomers as conjugation break spacers 

Ming-Han Chen, Yu-Chun Huang, Fu-En Szu, Jung-Yao Chen, Man-kit Leung, Yan-Cheng Lin 

 

  Enhancing charge transport in isoindigo-based donor–acceptor copolymers by combining ionic doping with polar alkoxy side chains 

Sheng Chuo, Yun-Ching Peng, Thanapon Puangniyom, Qun-Gao Chen, Chu-Chen Chueh,Wen-Ya Lee 

  Polymerized ionic liquid dielectrics tune molecular orientation and operating voltage in silicon phthalocyanine OTFTs 

Bahar Ronnasi, Nicolas Ledos, Benjamin King, Benoît H. Lessard 

 

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