Archive for the ‘Hot Articles’ Category

July’s HOT articles

Take a look at our HOT articles for July. These are only free to acess for 4 weeks only and are available for viewing in a collection on our website.

A mononuclear Ni(II) complex: a field induced single-molecule magnet showing two slow relaxation processes
Jozef Miklovič, Dušan Valigura, Roman Boča and Ján Titiš
Dalton Trans., 2015, 44, 12484-12487
DOI: 10.1039/C5DT01213A

Graphical Abstract

  

Free to access until 6th August 2015 

 


 ZnII and HgII binding to a designed peptide that accommodates different coordination geometries
Dániel Szunyogh, Béla Gyurcsik, Flemming H. Larsen, Monika Stachura, Peter W. Thulstrup, Lars Hemmingsen and Attila Jancsó
Dalton Trans., 2015, 44, 12576-12588
DOI: 10.1039/C5DT00945F 

Graphical Abstract 

Free to access until 6th August 2015  


 

Photophysical tuning of the aggregation-induced emission of a series of para-substituted aryl bis(imino)acenaphthene zinc complexes
Daniel A. Evans, Lucia Myongwon Lee, Ignacio Vargas-Baca and Alan H. Cowley
Dalton Trans., 2015, 44, 11984-11996
DOI: 10.1039/C5DT01529D 

Graphical Abstract

Free to access until 6th August 2015


An investigation into the photochemistry of, and the electrochemically induced CO-loss from, [(CO)5MC(OMe)Me](M = Cr or W) using low-temperature matrix isolation, picosecond infrared spectroscopy, cyclic voltammetry, and time-dependent density functional theory 
Suzanne McMahon, Saeed Amirjalayer, Wybren J. Buma, Yvonne Halpin, Conor Long, A. Denise Rooney, Sander Woutersen and Mary T. Pryce
Dalton Trans., 2015, Advance Article 
DOI: 10.1039/C5DT01568E

Graphical Abstract

Free to access until 6th August 2015


Aza-macrocyclic complexes of the Group 1 cations – synthesis, structures and density functional theory study
John Dyke, William Levason, Mark E. Light, David Pugh, Gillian Reid, Hanusha Bhakhoa, Ponnadurai Ramasami and Lydia Rhyman  
Dalton Trans., 2015, Advance Article  
DOI: 10.1039/C5DT01865J  

Graphical Abstract

Free to access until 6th August 2015


As-stereogenic C2-symmetric organoarsines: synthesis and enantioselective self-assembly into a dinuclear triple-stranded helicate with copper iodide
Hiroki Adachi, Hiroaki Imoto, Seiji Watase, Kimihiro Matsukawa and Kensuke Naka 
Dalton Trans., 2015, Advance Article  
DOI: 10.1039/C5DT01490E  

Graphical Abstract

Free to access until 6th August 2015

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New HOT articles

Take a look at our HOT articles for May. These are only free to acess for 4 weeks only and are available for viewing in a collection on our website

Synthesis of CuInS2 nanocrystals from a molecular complex – characterization of the orthorhombic domain structure
Jorge L. Cholula-Díaz, Gerald Wagner, Dirk Friedrich, Oliver Oeckler and Harald Krautscheid
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00419E

Graphical Abstract

 

Free to access until 30th June 2015


A cascade approach to hetero-pentanuclear manganese-oxide clusters in polyoxometalates and their single-molecule magnet properties
Kosuke Suzuki, Rinta Sato, Takuo Minato, Masahiro Shinoe, Kazuya Yamaguchi and Noritaka Mizuno
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT01363A

Graphical Abstract

 

Free to access until 30th June 2015


 

Quantum chemical and solution phase evaluation of metallocenes as reducing agents for the prospective atomic layer deposition of copper
Gangotri Dey, Jacqueline S. Wrench, Dirk J. Hagen, Lynette Keeney and Simon D. Elliott
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00922G

Graphical Abstract

Free to access until 16th June 2015


Synthesis of copper ion incorporated horseradish peroxidase-based hybrid nanoflowers for enhanced catalytic activity and stability
Burcu Somturk, Mehmet Hancer, Ismail Ocsoy and Nalan Özdemir
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT01250C

Graphical Abstract

Free to access until 16th June 2015


Platinum carbon bond formation via Cu(I) catalyzed Stille-type transmetallation: reaction scope and spectroscopic study of platinum-arylene complexes
Ali S. Gundogan, Xiangli Meng, Russell W. Winkel and Kirk S. Schanze
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00538H

Graphical Abstract

Free to access until 16th June 2015


Exceptionally rapid CO release from a manganese(I) tricarbonyl complex derived from bis(4-chloro-phenylimino)acenaphthene upon exposure to visible light
Samantha J. Carrington, Indranil Chakraborty and Pradip K. Mascharak
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT01007A

Graphical Abstract

Free to access until 16th June 2015


5-(Fluorodinitromethyl)-2H-tetrazole and its tetrazolates – Preparation and Characterization of New High Energy Compounds
Ralf Haiges and Karl O. Christe
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00291E 

Graphical Abstract

Free to access until 25th May 2015


Synthesis of magnesium ZIF-8 from Mg(BH4)2
S. Horike, K. Kadota, T. Itakura, M. Inukai and S. Kitagawa
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT01183C 

Graphical Abstract 

Free to access until 25th May 2015

 


16-Electron pentadienyl- and cyclopentadienyl-ruthenium half-sandwich complexes with bis(imidazol-2-imine) ligands and their use in catalytic transfer hydrogenation
Thomas Glöge, Kristof Jess, Thomas Bannenberg, Peter G. Jones, Nadine Langenscheidt-Dabringhausen, Albrecht Salzer and Matthias Tamm
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT01080B 

Graphical Abstract 

Free to access until 25th May 2015 


 

Structural and electronic characterization of multi-electron reduced naphthalene (BIAN) cobaloximes
Owen M. Williams, Alan H. Cowley and Michael J. Rose
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00924C 

Graphical Abstract 

Free to access until 25th May 2015

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March’s HOT articles

Take a look at HOT articles for March. These are only free to acess for 4 weeks only and are available for viewing in a collection on our website.

An ionic liquid process for mercury removal from natural gas
Mahpuzah Abai, Martin P. Atkins, Amiruddin Hassan, John D. Holbrey, Yongcheun Kuah, Peter Nockemann, Alexander A. Oliferenko, Natalia V. Plechkova, Syamzari Rafeen, Adam A. Rahman, Rafin Ramli, Shahidah M. Shariff, Kenneth R. Seddon, Geetha Srinivasan and Yiran Zou  
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03273J

Graphical Abstract

Free to access until 24th April 2015


Relationship between crystal structure and thermo-mechanical properties of kaolinite clay: beyond standard density functional theory
Philippe F. Weck, Eunja Kim and Carlos F. Jové-Colón 
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00590F

Graphical Abstract

Free to access until 23rd April 2015


The titanium tris-anilide cation [Ti(N[tBu]Ar)3]+ stabilized as its perfluoro-tetra-phenylborate salt: structural characterization and synthesis in connection with redox activity of 4,4′-bipyridine dititanium complexes
Heather A. Spinney, Christopher R. Clough and Christopher C. Cummins
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00105F

Graphical Abstract

Free to access until 14th April 2015


Iridium–bipyridine periodic mesoporous organosilica catalyzed direct C–H borylation using a pinacolborane
Yoshifumi Maegawa and Shinji Inagaki
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C5DT00239G

Graphical Abstract

Free to access until 14th April 2015

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A Cagey Conundrum

“My original intention in the late 1940s was to spend a few years understanding the boranes, and then to discover a systematic valence description of the vast numbers of electron deficient intermetallic compounds. I have made little progress toward this latter objective,” said the late Professor William N. Lipscomb in his 1976 Nobel acceptance speech.1

In their recent Dalton Transactions Hot Article, Jose M. Goicoechea and John E. McGrady examine the chemistry of main group cluster-encapsulated transition metal atoms, laying another piece of the foundation of Lipscomb’s “latter objective.”

The authors assign themselves an ambitious task: to provide a system to predict the geometries of cages of the tetrel elements (C, Si, Ge, Sn, Pb) which encapsulate transition metal atoms.  They focus on six high-symmetry cage structures, shown below, which have been observed for tetrel-encapsulated metal atoms (denoted M@Ex, for example Ni@Ge12.).

The six three-dimensional cage geometries examined.

Lipscomb’s elegantly-described closo, nido, and arachno borane structures (“closed,”“nest”, and “spider’s web,” respectively) provided an initial basis for classifications of cages.  Later, the Wade/Mingos rules laid the foundation for predicting the geometries based on the electronic structure of the cluster.

Goicoechea and McGrady use the total valence electron count –  of the tetrel cages, plus the d-electron count of the encapsulated metal – to describe patterns in the structures.  Nevertheless, some results defy electron-count classification, for example, the preference of silicon cages to form D6h-symmetric hexagonal prisms in M@Si12 complexes, in contrast to the M@Ge12 analogues.

It is a broad, big-picture paper, a synthesis of a wide range of experimental and theoretical results.  Some structures are known experimentally from x-ray crystallography, some have only been predicted computationally.  The authors discuss the varying relevance of considering the d-electron counts of the metals, and technological implications such as quenching of the magnetic moment of encapsulated metal atoms.  For me, the scope alone made this a worthwhile read.

Read the full article now:

On the structural landscape in endohedral silicon and germanium clusters, M@Si12 and M@Ge12
José M. Goicoechea and John E. McGrady
Dalton Trans., 2015, DOI: 10.1039/C4DT03573A

1 Lipscomb, W.N. “The Boranes and Their Relatives” in Les Prix Nobel en 1976. Imprimerie Royal PA Norstedt & Soner, Stockholm, 1977


Ian Mallov Ian Mallov is currently a Ph.D. student in Professor Doug Stephan’s group at the University of Toronto. His research is focused on synthesizing new Lewis-acidic compounds active in Frustrated Lewis Pair chemistry. He grew up in Truro, Nova Scotia and graduated from Dalhousie University and the University of Ottawa, and worked in chemical analysis in industry for three years before returning to grad school.
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February’s HOT articles

This month brings some more HOT articles. These are only free to acess for 4 weeks only and are available for viewing on our website.

Thermoelectric properties of the Zintl phases Yb5M2Sb6 (M = Al, Ga, In)
Umut Aydemir, Alex Zevalkink, Alim Ormeci, Heng Wang, Saneyuki Ohno, Sabah Bux and G. Jeffrey Snyder
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03773A

Graphical Abstract

Free to access until 25th March 2015


Exploring excited states of Pt(II) diimine catecholates for photoinduced charge separation
Paul A. Scattergood, Patricia Jesus, Harry Adams, Milan Delor, Igor V. Sazanovich, Hugh D. Burrows, Carlos Serpa and Julia A. Weinstein
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03466J

Graphical Abstract

Free to access until 25th March 2015


On the structural landscape in endohedral silicon and germanium clusters, M@Si12 and M@Ge12
José M. Goicoechea and John E. McGrady
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03573A

Graphical Abstract

Free to access until 9th March 2015


The synthesis, structure, topology and catalytic application of a novel cubane-based copper(II) metal–organic framework derived from a flexible amido tripodal acid
Anirban Karmakar, Clive L. Oliver, Somnath Roy and Lars Öhrström
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03087G

Graphical Abstract

Free to access until 9th March 2015

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January’s HOT articles

A new year has brought a new crop of HOT articles for the month. As always, these are free to access for 4 weeks!

Our HOT articles have also been compiled into a collection and are available for viewing on our website.

Methylated Re(I) tetrazolato complexes: photophysical properties and Light Emitting Devices
Melissa V. Werrett, Gregory S. Huff, Sara Muzzioli, Valentina Fiorini, Stefano Zacchini, Brian W. Skelton, Antonio Maggiore, Joanna M. Malicka, Massimo Cocchi, Keith C. Gordon, Stefano Stagni and Massimiliano Massi
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03228D

Graphical Abstract

Free to access until 26th February 2015


Recent advances towards the fabrication and biomedical applications of responsive polymeric assemblies and nanoparticle hybrid superstructures
Xianglong Hu and Shiyong Liu
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03609C

Graphical Abstract

 

Free to access until 26th February 2015


Synthesis and characterization of substituted Schiff-base ligands and their d10 metal complexes: structure-induced luminescence tuning behaviors and applications in co-sensitized solar cells
Yu-Wei Dong, Rui-Qing Fan, Ping Wang, Li-Guo Wei, Xin-Ming Wang, Hui-Jie Zhang, Song Gao, Yu-Lin Yang and Yu-Lei Wang
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03602F

Graphical Abstract

Free to access until 26th February 2015

 


Spin-crossover behaviors in solvated cobalt(II) compounds
Shinya Hayami, Manabu Nakaya, Hitomi Ohmagari, Amolegbe Saliu Alao, Masaaki Nakamura, Ryo Ohtani, Ryotaro Yamaguchi, Takayoshi Kuroda-Sowa and Jack K. Clegg
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03743J

Graphical Abstract

 

Free to access until 26th February 2015

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December’s HOT articles

Enjoy a read of our end of year HOT articles which are free to access for 4 weeks only!

Our HOT articles have also been compiled into a collection and are available for viewing on our website.

A theoretical study of the aromaticity in neutral and anionic borole compounds
J. Oscar C. Jimenez-Halla, Eduard Matito, Miquel Solà, Holger Braunschweig, Christian Hörl, Ivo Krummenacher and Johannes Wahler
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03445G

Graphical Abstract 

Free to access until 6th February 2015


High performing smart electrochromic device based on honeycomb nanostructured h-WO3 thin films: hydrothermal assisted synthesis
Vijay V. Kondalkar, Sawanta S. Mali, Rohini R. Kharade, Kishorkumar V. Khot, Pallavi B. Patil, Rahul M. Mane, Sipra Choudhury, Pramod S. Patil, Chang K. Hong, Jin H. Kim and Popatrao N. Bhosale
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02953D

Graphical Abstract

Free to access until 6th February 2015


Application of three-coordinate copper(I) complexes with halide ligands in organic light-emitting diodes that exhibit delayed fluorescence
Masahisa Osawa, Mikio Hoshino, Masashi Hashimoto, Isao Kawata, Satoshi Igawa and Masataka Yashima
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02853H

Graphical Abstract

Free to access until 6th January 2015


Na0.3WO3 nanorods: a multifunctional agent for in vivo dual-model imaging and photothermal therapy of cancer cells
Yuxin Zhang, Bo Li, Yunjiu Cao, Jinbao Qin, Zhiyou Peng, Zhiyin Xiao, Xiaojuan Huang, Rujia Zou and Junqing Hu
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02927E

 

Graphical Abstract

Free to access until 6th January 2015


Transmetalation from B to Rh in the course of the catalytic asymmetric 1,4-addition reaction of phenylboronic acid to enones: a computational comparison of diphosphane and diene ligands
You-Gui Li, Gang He, Hua-Li Qin and Eric Assen B. Kantchev
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03147D

 

Graphical Abstract

Free to access until 1st January 2015


A contribution to the rational design of Ru(CO)3Cl2L complexes for in vivo delivery of CO
João D. Seixas, Marino F. A. Santos, Abhik Mukhopadhyay, Ana C. Coelho, Patrícia M. Reis, Luís F. Veiros, Ana R. Marques, Nuno Penacho, Ana M. L. Gonçalves, Maria J. Romão, Gonçalo J. L. Bernardes, Teresa Santos-Silva and   Carlos C. Romão
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02966F

Graphical Abstract

 

Free to access until 1st January 2015

 

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November’s HOT articles

Enjoy a read of our latest HOT articles which are free to access for 4 weeks only! 

Our HOT articles have also been compiled into a collection and are available for viewing on our website. 

Redox activity and π bonding in a tripodal seven-coordinate molybdenum(VI) tris(amidophenolate)
Travis Marshall-Roth and Seth N. Brown
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02936D 

 

Graphical Abstract 

Free to access until 28th December 2014 


FIrpic: archetypal blue phosphorescent emitter for electroluminescence
Etienne Baranoff and Basile F. E. Curchod
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02991G

Graphical Abstract 

Free to access until 28th December 2014


Optimizing the high-field relaxivity by self-assembling of macrocyclic Gd(III) complexes
Dale Lawson, Alessandro Barge, Enzo Terreno, David Parker, Silvio Aime and Mauro Botta
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02971B

Graphical Abstract

 

Free to access until 28th December 2014


 

Copper(I), silver(I) and gold(I) complexes of N-heterocyclic carbene-phosphinidene
Venkata A. K. Adiraju, Muhammed Yousufuddin and H. V. Rasika Dias
Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT03285C

Graphical Abstract

Free to access until 28th December 2014

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October’s HOT articles

Enjoy a read of our latest HOT articles which are free to access for 4 weeks only!

Our HOT articles have also been compiled into a collection and are available for viewing on our website.

A strong steric hindrance effect on ground state, excited state, and charge separated state properties of a CuI-diimine complex captured by X-ray transient absorption spectroscopy
J. Huang, M. W. Mara, A. B. Stickrath, O. Kokhan, M. R. Harpham, K. Haldrup, M. L. Shelby, X. Zhang, R. Ruppert, J.-P. Sauvage and L. X. Chen
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02046D

Graphical Abstract

Free to access until 26th November 2014


On the coordination chemistry of organochalcogenolates RNMe2^Eand RNMe2^E^O(E = S, Se) onto lead(II) and lighter divalent tetrel elements
Alexandra Pop, Lingfang Wang, Vincent Dorcet, Thierry Roisnel, Jean-François Carpentier, Anca Silvestru and Yann Sarazin
Dalton Trans., 2014, 43, 16459-16474
DOI: 10.1039/C4DT02252A

Graphical Abstract

Free to access until 26th November 2014


Niobium(V) and tantalum(V) halide chalcogenoether complexes – towards single source CVD precursors for ME2 thin films
Sophie L. Benjamin, Yao-Pang Chang, Chitra Gurnani, Andrew L. Hector, Michelle Huggon, William Levason and Gillian Reid
Dalton Trans., 2014, 43, 16640-16648
DOI: 10.1039/C4DT02694B

Graphical Abstract

Free to access until 26th November 2014


The crystal structure of paramagnetic copper(II) oxalate (CuC2O4): formation and thermal decomposition of randomly stacked anisotropic nano-sized crystallites
Axel Nørlund Christensen, Bente Lebech, Niels Hessel Andersen and Jean-Claude Grivel
Dalton Trans., 2014, 43, 16754-16768
DOI: 10.1039/C4DT01689K

Graphical Abstract

Free to access until 26th November 2014


Lithiated sulfoxides: α-sulfinyl functionalized carbanions
Gerd Ludwig, Tobias Rüffer, André Hoppe, Till Walther, Heinrich Lang, Stefan G. Ebbinghaus and Dirk Steinborn
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02238F

Graphical Abstract

Free to access until 26th November 2014


Encapsulation of large dye molecules in hierarchically superstructured metal–organic frameworks
Yanfeng Yue, Andrew J. Binder, Ruijing Song, Yuanjing Cui, Jihua Chen, Dale K. Hensley and Sheng Dai
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02516D

Graphical Abstract

Free to access until 26th November 2014

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September’s HOT articles

Enjoy a read of Autumn’s crop of HOT articles which are free to access for 4 weeks only!

Our HOT articles have also been compiled into a collection and are available for viewing on our website.

Metal-mediated coupling of amino acid esters with isocyanides leading to new chiral acyclic aminocarbene complexes
Tatyana B. Anisimova, M. Fátima C. Guedes da Silva, Vadim Yu. Kukushkin, Armando J. L. Pombeiro and Konstantin V. Luzyanin
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT01917B

Graphical Abstract

Free to access until 27th October 2014


Photoinduced hydrogen evolution by a pentapyridine cobalt complex: elucidating some mechanistic aspects
Elisa Deponti, Alessandra Luisa, Mirco Natali, Elisabetta Iengo and Franco Scandola
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02269F

Graphical Abstract

Free to access until 27th October 2014


Efficient halogen photoelimination from dibromo, dichloro and difluoro tellurophenes
Elisa I. Carrera and Dwight S. Seferos
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT01751J

Graphical Abstract

Free to access until 17th October 2014


Synthesis, structure and catalytic activity of a gold(I) complex containing 1,2-bis(diphenylphosphino)benzene monoxide
Christine Hahn, Leticia Cruz, Amanda Villalobos, Liliana Garza and Samuel Adeosun
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02116A

Graphical Abstract

Free to access until 17th October 2014


1,3,5-Triferrocenyl-2,4,6-tris(ethynylferrocenyl)-benzene – a new member of the family of multiferrocenyl-functionalized cyclic systems
Ulrike Pfaff, Grzegorz Filipczyk, Alexander Hildebrandt, Marcus Korb and Heinrich Lang
Dalton Trans., 2014, Advance Article
DOI: 10.1039/C4DT02307B

Graphical Abstract

Free to access until 17th October 2014

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